Is regional air quality model diversity representative of uncertainty for ozone simulation ?

Robert Vautard 1 M. van Loon 2 M. Schaap 3 R. Bergstrom 4 Bertrand Bessagnet 5 J. Brandt 6 P. Builtjes 3 J.H. Christensen 6 C. Cuvelier 7 A. Graff 8 J.E. Jonson 2 M. Krol 9 J. Langner 4 P. Roberts 10 Laurence Rouil 5 R. Stern 11 L. Tarrason 2 P. Thunis 7 E. Vignati 7 L. White 12 Philippe Wind 2
1 LSCE - Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette]
2 MSC-W - EMEP Meteorological Synthesizing Centre-West
3 TNO - The Netherlands Organisation for Applied Scientific Research
4 SMHI - Swedish Meteorological and Hydrological Institute
5 INERIS - Institut National de l'Environnement Industriel et des Risques
6 National Environment Research Institute
7 IES - JRC Institute for Environment and Sustainability
8 Übergreifende Angelegenheiten der Luftreinhaltung
9 Institute of Marine and Atmospheric Research
10 Shell Global / HSE Department
11 Institut für Meteorologie [Berlin]
12 Conservation of Clean Air and Water in Europe
Abstract : We examine whether seven state-of-the-art European regional air quality models provide daily ensembles of predicted ozone maxima that encompass observations. Using tools borrowed from the evaluation of ensemble weather forecasting, we analyze statistics of simulated ensembles of ozone daily maxima over an entire summer season. Although the model ensemble overestimates ozone, the distribution of simulated concentrations is representative of the uncertainty. The spread of simulations is due to random fluctuations resulting from differences in model formulations and input data, but also to the spread between individual model systematic biases. The ensemble average skill increases as the spread decreases. The skill of the ensemble in giving probabilistic predictions of threshold exceedances is also demonstrated. These results allow for optimism about the ability of this ensemble to simulate the uncertainty of the impact of emission control scenarios.
Keywords : ATMOSPHERIC COMPOSITION AND STRUCTURE : POLLUTION : URBAN AND REGIONAL : ATMOSPHERIC COMPOSITION AND STRUCTURE : TROPOSPHERE : CONSTITUENT TRANSPORT AND CHEMISTRY ATMOSPHERIC COMPOSITION AND STRUCTURE : POLLUTION : URBAN AND REGIONAL : ATMOSPHERIC COMPOSITION AND STRUCTURE : TROPOSPHERE : CONSTITUENT TRANSPORT AND CHEMISTRY.
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Journal articles
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Submitted on : Friday, March 21, 2014 - 2:11:03 PM
Last modification on : Wednesday, February 27, 2019 - 11:08:02 AM

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Robert Vautard, M. van Loon, M. Schaap, R. Bergstrom, Bertrand Bessagnet, et al.. Is regional air quality model diversity representative of uncertainty for ozone simulation ?. Geophysical Research Letters, American Geophysical Union, 2006, 33 (24), pp.art n° L24818. ⟨10.1029/2006GL027610⟩. ⟨ineris-00963044⟩

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